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Feb 2016
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ZHANG Hao, ZHU Feng-sen, LI Xiao-dong, WU Ang-jian, BO Zheng, CEN Ke-fa. Rotating gliding arc plasma assisted hydrogen production from methane decomposition in argon[J]. JOURNAL OF MECHANICAL ENGINEERING, 2016, 44(2): 192-200.
Citation: ZHANG Hao, ZHU Feng-sen, LI Xiao-dong, WU Ang-jian, BO Zheng, CEN Ke-fa. Rotating gliding arc plasma assisted hydrogen production from methane decomposition in argon[J]. JOURNAL OF MECHANICAL ENGINEERING, 2016, 44(2): 192-200.

Rotating gliding arc plasma assisted hydrogen production from methane decomposition in argon

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  • Corresponding author: Tel: 0571-87952037, Fax: 0571-87952438, E-mail: lixd@zju.edu.cn
  • Received Date: 09 Jun 2015
  • Rev Recd Date: 14 Sep 2015
  • A kind of rotating gliding arc (RGA) argon plasma co-driven by tangential flow and magnetic field was investigated and used for hydrogen production from methane decomposition.In order to obtain insights into the physical characteristics of the RGA plasma, optical emission spectroscopy (OES) analysis was used to determine the electron temperature and electron density.In addition, the effects of feed flow rate and CH4/Ar ratio on the performance of the methane decomposition process in this RGA plasma were also investigated.Results have shown that, the RGA plasma is a kind of unique plasma between thermal and non-thermal plasma, with electron temperature of 1.0-2.0 eV and electron density of 1015 cm-3.In this system, the CH4 conversion could be 22.1%-70.2% and it increased with the increase of flow rate or CH4/Ar ratio.The H2 selectivity varied from 21.2% to 61.2%, and with the augment of flow rate, the H2 selectivity first varied slightly and then increased.A comparison of different non-thermal plasmas (e.g., microwave, radio frequency, and dielectric barrier discharge) showed that the RGA plasma could provide a relatively high CH4 conversion and H2 selectivity, as well as a relatively low energy consumption for H2 production, while maintaining a high flow rate (i.e., processing capacity) of 6-20 L/min.

     

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