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利用数值模拟研究表面增强相干反斯托克斯拉曼散射增强基底

李健康 李睿

李健康, 李睿. 利用数值模拟研究表面增强相干反斯托克斯拉曼散射增强基底[J]. 机械工程学报, 2021, 70(10): 104207. doi: 10.7498/aps.70.20201773
引用本文: 李健康, 李睿. 利用数值模拟研究表面增强相干反斯托克斯拉曼散射增强基底[J]. 机械工程学报, 2021, 70(10): 104207. doi: 10.7498/aps.70.20201773
Li Jian-Kang, Li Rui. Numerical simulation study of surface enhancement coherent anti-Stokes Raman scattering reinforced substrate[J]. JOURNAL OF MECHANICAL ENGINEERING, 2021, 70(10): 104207. doi: 10.7498/aps.70.20201773
Citation: Li Jian-Kang, Li Rui. Numerical simulation study of surface enhancement coherent anti-Stokes Raman scattering reinforced substrate[J]. JOURNAL OF MECHANICAL ENGINEERING, 2021, 70(10): 104207. doi: 10.7498/aps.70.20201773

利用数值模拟研究表面增强相干反斯托克斯拉曼散射增强基底

doi: 10.7498/aps.70.20201773
详细信息
    通讯作者:

    E-mail: rli@dlut.edu.cn

  • 中图分类号: 42.65.Dr, 71.45.Gm, 52.38.Bv

Numerical simulation study of surface enhancement coherent anti-Stokes Raman scattering reinforced substrate

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  • 摘要: 为表面增强相干反斯托克斯拉曼散射(surface enhancement coherent anti-Stokes Raman scattering, SECARS)提供具有高增强、稳定性好的等离激元增强基底是十分重要的. 本文从实际出发, 在理论上设计了一种新的SECARS基底, 其可以利用结构自身的杂化共振与额外激发的电荷转移等离子体共振相互作用产生Fano共振, 并通过调节电荷转移等离子体共振来改变Fano共振的波长位置. 通过对L-色氨酸1557 cm–1处的拉曼模式的数值模拟得到的数据表明, 这种具有空间对称性的结构可以产生多个不依赖入射光偏振方向的高增强热点, 这些热点处的信号相对于普通相干反斯托克斯拉曼散射(coherent anti-Stokes Raman scattering, CARS)信号, 其增强因子普遍可以达到1012, 最大处可达到1014. 这种利用电荷转移等离子体来设计基底的方法可以在SECARS的实用性基底中得到应用并为其他非线性光学工艺的设计提供了新的思路.

     

  • 图  基底的结构示意图 (a)与其对应的参数示意图(b)

    Figure  1.  Sketch of the structure(a) with the defined parameters and coordinate axis(b).

    图  圆盘的参数不变(r1 = 63 nm, r2 = 97 nm, d = 10 nm, h1 = 50 nm)改变导电结参数时散射系数的变化 (a) $ \theta $ = 450, h2 = 50 nm, O(x, y) = (100, 100), 改变结的宽度l从30到50 nm; (b) l = 40 nm, h2 = 50 nm, O(x, y) = (100, 100), 改变倾斜角度 $ \theta $ 从250到450; (c) l = 40 nm, $ \theta $ = 450, h2 = 50 nm, 改变中心坐标O(x, y)从(70, 70)到(110, 110); (d) l = 40 nm, $ \theta $ = 450, O(x, y) = (100, 100), 改变结厚度h2从30到50 nm

    Figure  2.  When the parameters of the disc are unchanged (r1 = 63 nm, r2 = 97 nm, d = 10 nm, h1 = 50 nm) that the scattering spectrum depond on geometrical parameters: (a) Vary l with $ \theta $ = 450, h2 = 50 nm, O(x, y) = (100, 100); (b) vary $ \theta $ with l = 40 nm, h2 = 50 nm, O(x, y) = (100, 100); (c) vary O(x, y) with l = 40 nm, $ \theta $ = 450, h2 = 50 nm; (d) vary $ {h}_{2} $ with l = 40 nm, $ \theta $ = 450, O(x, y) = (100, 100).

    图  入射光不同偏振角度时的相同参数(l = 35 nm, h2 = 50 nm, O(x, y) = (100, 100), r1 = 63 nm, r2 = 97 nm, d = 10 nm)结构的散射系数, 偏振角度定义为入射光偏振方向与结构Y轴夹角

    Figure  3.  . Scattering spectra for various excitation polarizations with the same parameters (l = 35 nm, h2 = 50 nm, O(x, y) = (100, 100), r1 = 63 nm, r2 = 97 nm, d = 10 nm), and the polarization angle is defined as the angle between the polarization direction and the Y-axis.

    图  (a) 入射光偏振方向沿基底的Y轴方向时与入射光偏振方向与基底的Y轴的夹角为450时基底表面912 nm, 1064 nm, 1275 nm三个波长处与1064 nm时基底中心YZ横截面处的电场强度空间分布; (b) 当入射光偏振方向沿基底的Y轴方向夹角θ为0°, 15°, 30°, 45°时基底表面对应的增强GSECARS因子的对数空间分布图

    Figure  4.  (a)The spatial distributions of enhanced electric-filed amplitude (|E/E0|) in the top surface plane of the structure at three characteristic wavelengths for two polarizations; (b) the corresponding SECARS map for various polarizations. From the top to bottom, the polarization angle θ equals to 0°, 15°, 30°, 45°, respectively.

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出版历程
  • 收稿日期:  2020-10-24
  • 修回日期:  2020-11-20
  • 网络出版日期:  2021-05-27
  • 发布日期:  2021-05-27

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